Transforming Fossil Fuels into Heat or Hydrogen

Greenhouse gases, in particular CO2 are the main cause of climate change. This project was motivated by finding an alternative way of using natural gas to produce heat for industrial facilities with reduced CO2 production. The main purpose of this project was to investigate pyrolysis of natural gas with a medium-scale set-up (8 kw). Natural gas can be decomposed into hydrogen and carbon black at high temperatures.


Hydrogen can be used as a clean fuel and carbon black is a valuable raw material for many industries such as tire, rubber, ink and pigments.


Two natural gas thermal decomposition systems will be investigated in order to transform fossil fuels into either heat or hydrogen:


1) Gas-phase pyrolysis, where the heat for pyrolysis is provided by burning natural gas and the pyrolysis occurs via heat transfer from the gas-phase products of combustion.


2) Gas-phase pyrolysis, where the heat for pyrolysis is provided by electricity and the pyrolysis occurs via heat transfer through a conductive surface.

A Reduced Methane Pyrolysis Mechanism for Above-Atmospheric Pressure Conditions

Jason Scott Olfert, Marc Secanell, Larry William Kostiuk, Ambuj Punia

Peer-Reviewed Journal Article

Analysis of the products and kinetic rates of methane thermal decomposition. Part II: Numerical models

Jason Scott Olfert, Marc Secanell, Larry William Kostiuk, Ambuj Punia

Conference Proceedings

Analysis of the products and kinetic rates of methane thermaldecomposition. Part I: Experimental apparatus

Jason Scott Olfert, Marc Secanell, Larry William Kostiuk, Ambuj Punia

Conference Proceedings

Characterization of particles generated by non-catalytic methane pyrolysis in a tubular flow reactor

Jason Scott Olfert, Marc Secanell, Natalia Semagina, Jing Shen, Ehsan Abbasi Atibeh, Arash Naseri

Peer-Reviewed Journal Article

Dataset of methane pyrolysis products in a batch reactor as a function of time at high temperatures and pressures

Jason Scott Olfert, Marc Secanell, Larry William Kostiuk, Ambuj Punia

Peer-Reviewed Journal Article

Effects of Co-flow on Jet Diffusion Flames: Flow Field and Emissions

Doctoral Thesis/Dissertation

Experimental Investigation of Carbon Black Properties Produced by the Thermal Decomposition of Methane in the Products of Premixed Flames

Master Thesis

Experimental and numerical analysis of a methane thermal decomposition reactor

Marc Secanell, Larry William Kostiuk

Peer-Reviewed Journal Article

Experimental and numerical analysis of methane pyrolysis at elevated pressure

Jason Scott Olfert, Marc Secanell, Larry William Kostiuk, Ambuj Punia

Peer-Reviewed Journal Article

Experimental study of methane decarbonization to produce hydrogen using a laminar premixed flame

Master Thesis

Hydrogen research heats up

Jason Scott Olfert

Interview (Broadcast or Text)

Kinetics of methane pyrolysis: An optimized mechanism

Jason Scott Olfert, Marc Secanell, Larry William Kostiuk, Ambuj Punia

Conference Proceedings

Measurements of Methane Pyrolysis in a Constant Volume Batch Reactor at High Temperatures and Pressures Author / Creator

Master Thesis

Nanoparticle Emission Characteristics during Methane Pyrolysis in a Laminar Premixed Flame

Jason Scott Olfert, Larry William Kostiuk

Conference/Symposium/Workshop Contribution

New hydrogen production method

Jason Scott Olfert

Interview (Broadcast or Text)

New research exploring more environmentally friendly ways to extract hydrogen,

Jason Scott Olfert

Interview (Broadcast or Text)

Preliminary experimental study of methane decarbonization using a laminar premixed flame

Jason Scott Olfert, Larry William Kostiuk

Conference Proceedings

Properties of carbon black produced by the thermal decomposition of methane in the products of premixed flames

Jason Scott Olfert, Larry William Kostiuk

Peer-Reviewed Journal Article

Properties of carbon particles generated by methane decarbonization in oxygen deficient gas streams

Jason Scott Olfert, Larry William Kostiuk

Conference Proceedings

U of A researchers at forefront of the province's hydrogen future

Jason Scott Olfert

Interview (Broadcast or Text)