Understanding and modelling black carbon formation

Micron and sub-micron scale black carbon particulates are a relatively short-lived climate airborne pollutants (though their deposition on arctic ice can have longer term impacts) that is seen by many as the second most important class of anthropogenic climate forcing materials, behind carbon dioxide. Its origins are directly attributable to combustion of hydrocarbons and coal.


Most controlled combustion systems, such as vehicles and power plants, have black carbon mitigation strategies. Some exceptions continue to struggle in this regard. For example, marine transport and bio-derived fuels used in commercial aircraft. There are also uncontrolled combustion systems that are seen as the biggest emitters of black carbon, and these include the natural processes of wildfires (in particular, smoldering combustion) or the industrial process of flaring.


The objective of this project is to understand and model the fundamentals of black carbon formation that can be applied in combustion or pyrolysis situations in order to either mitigate their emissions or to form and capture the black carbon into a valuable material.

Analysis of the products and kinetic rates of methane thermal decomposition. Part II: Numerical models

Jason Scott Olfert, Marc Secanell, Larry William Kostiuk, Ambuj Punia, James Kole William Tatum

Conference Proceedings

Analysis of the products and kinetic rates of methane thermaldecomposition. Part I: Experimental apparatus

Jason Scott Olfert, Marc Secanell, Larry William Kostiuk, Ambuj Punia, James Kole William Tatum

Conference Proceedings

Biobattery concept: Decentralized production of fuel from forest biomass, agriculture residue and municipal solid waste

Amit Kumar, Raj Gupta, Larry William Kostiuk, Vinoj Kurian, Wasel-ur Rahman

Conference/Symposium/Workshop Contribution

Dataset of methane pyrolysis products in a batch reactor as a function of time at high temperatures and pressures

Jason Scott Olfert, Marc Secanell, Larry William Kostiuk, Ambuj Punia, James Kole William Tatum

Peer-Reviewed Journal Article

Decentralized use of forest biomass, agricultural residue, and municipal solid waste through the biobattery concept

Amit Kumar, Raj Gupta, Larry William Kostiuk, Vinoj Kurian

Conference/Symposium/Workshop Contribution

Experimental and numerical analysis of a methane thermal decomposition reactor

Marc Secanell, Larry William Kostiuk

Peer-Reviewed Journal Article

Kinetics of methane pyrolysis: An optimized mechanism

Jason Scott Olfert, Marc Secanell, Larry William Kostiuk, Ambuj Punia, James Kole William Tatum

Conference Proceedings

Nanoparticle Emission Characteristics during Methane Pyrolysis in a Laminar Premixed Flame

Jason Scott Olfert, Larry William Kostiuk, Mohammad Afroughi, Farjad Falahati

Conference/Symposium/Workshop Contribution

Preliminary experimental study of methane decarbonization using a laminar premixed flame

Jason Scott Olfert, Larry William Kostiuk, Mohammad Afroughi, Farjad Falahati

Conference Proceedings

Properties of carbon black produced by the thermal decomposition of methane in the products of premixed flames

Jason Scott Olfert, Larry William Kostiuk, Mohammad Afroughi, Farjad Falahati

Peer-Reviewed Journal Article

Properties of carbon particles generated by methane decarbonization in oxygen deficient gas streams

Jason Scott Olfert, Larry William Kostiuk, Mohammad Afroughi, Farjad Falahati

Conference Proceedings